Femtosecond coherent nano-spectroscopy of coupled molecular dynamics

  • Joanna M. Atkin
  • , Paul M. Sass
  • , Honghua U. Yang
  • , Paul Teichen
  • , Joel Eaves
  • , Markus B. Raschke

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

We isolate the vibrational free-induction decay of a homogeneous molecular subensemble using ultrafast infrared vibrational scattering-scanning near-field microscopy. The observed long-lived few picosecond vibrational coherences, intramolecular coherence transfer, and spatial variations in vibrational modes indicate non-ergodic behavior. © OSA 2015.
Original languageEnglish
Title of host publicationCLEO: QELS - Fundamental Science, CLEO_QELS 2015
Volume2015-
DOIs
StatePublished - 2015

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