Abstract
We isolate the vibrational free-induction decay of a homogeneous molecular subensemble using ultrafast infrared vibrational scattering-scanning near-field microscopy. The observed long-lived few picosecond vibrational coherences, intramolecular coherence transfer, and spatial variations in vibrational modes indicate non-ergodic behavior. © OSA 2015.
| Original language | English |
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| Title of host publication | CLEO: QELS - Fundamental Science, CLEO_QELS 2015 |
| Volume | 2015- |
| DOIs | |
| State | Published - 2015 |